Abstract
An orphan radium-beryllium (Ra–Be) neutron source (Nuclear Chicago Corporation) detected inside a scrap metal shipping container, was seized and subjected to nuclear forensic analysis. Physical and chemical characterization methods were used before and after source dismantling. Non-Destructive Testing (NDT) proved to be most useful for initial analysis of the source. Dissolution of the Ra-Be capsule was followed with elemental analysis by Inductively Coupled Plasma (ICP) Atomic Emission Spectroscopy (AES) and Mass Spectrometry (MS). Model age determination by ICP-MS (81.6 y ± 4.08) was found to be sensitive to insufficient accuracy in measuring daughters present in the parent solution.
| Original language | English |
|---|---|
| Pages (from-to) | 51-60 |
| Number of pages | 10 |
| Journal | Journal of Radioanalytical and Nuclear Chemistry |
| Volume | 329 |
| Issue number | 1 |
| DOIs | |
| State | Published - 1 Jul 2021 |
| Externally published | Yes |
Keywords
- Neutron radiography
- Nuclear forensics
- Ra-Be neutron source
- Radio-chronometry
- X-ray radiography
ASJC Scopus subject areas
- Analytical Chemistry
- Nuclear Energy and Engineering
- Radiology Nuclear Medicine and imaging
- Pollution
- Spectroscopy
- Public Health, Environmental and Occupational Health
- Health, Toxicology and Mutagenesis
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