Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)

Russell Cooper; Igor Rahinov; Cheng Yuan; Xueming Yang; Daniel J. Auerbach; Alec M. Wodtke

doi:10.1116/1.3071971

Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)

Russell Cooper, Igor Rahinov, Cheng Yuan, Xueming Yang, Daniel J. Auerbach, Alec M. Wodtke

Research output: Contribution to journal › Article › peer-review

27 Scopus citations

Abstract

The authors report high resolution state resolved measurements of the translational inelasticity of HCl (v=0→0,J=0→4) colliding with a Au(111) surface at near normal incidence in the energy range of 0.28-1.27 eV. The translational inelasticity is large and indistinguishable from previous measurements for the HCl (v=2→2,J=1→5) channel. They discuss these observations in terms of an impulse approximation as well as the possible role of translational excitation of electron-hole pairs in the solid.

Original language	English
Pages (from-to)	907-912
Number of pages	6
Journal	Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films
Volume	27
Issue number	4
DOIs	https://doi.org/10.1116/1.3071971
State	Published - 17 Jul 2009
Externally published	Yes

ASJC Scopus subject areas

Condensed Matter Physics
Surfaces and Interfaces
Surfaces, Coatings and Films

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Cooper, R., Rahinov, I., Yuan, C., Yang, X., Auerbach, D. J., & Wodtke, A. M. (2009). Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111). Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films, 27(4), 907-912. https://doi.org/10.1116/1.3071971

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title = "Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)",

abstract = "The authors report high resolution state resolved measurements of the translational inelasticity of HCl (v=0→0,J=0→4) colliding with a Au(111) surface at near normal incidence in the energy range of 0.28-1.27 eV. The translational inelasticity is large and indistinguishable from previous measurements for the HCl (v=2→2,J=1→5) channel. They discuss these observations in terms of an impulse approximation as well as the possible role of translational excitation of electron-hole pairs in the solid.",

author = "Russell Cooper and Igor Rahinov and Cheng Yuan and Xueming Yang and Auerbach, {Daniel J.} and Wodtke, {Alec M.}",

note = "Funding Information: The authors gratefully acknowledge the financial support from the Department of Energy Office of Basic Energy Sciences, under Grant No. DE-FG02-03ER15441 as well as the Partnership for International Research and Education—for Electronic Chemistry and Catalysis at Interfaces—NSF Grant No. OISE-0530268.",

year = "2009",

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day = "17",

doi = "10.1116/1.3071971",

language = "English",

volume = "27",

pages = "907--912",

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Cooper, R, Rahinov, I, Yuan, C, Yang, X, Auerbach, DJ & Wodtke, AM 2009, 'Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)', Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films, vol. 27, no. 4, pp. 907-912. https://doi.org/10.1116/1.3071971

Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111). / Cooper, Russell; Rahinov, Igor; Yuan, Cheng et al.
In: Journal of Vacuum Science and Technology A: Vacuum, Surfaces and Films, Vol. 27, No. 4, 17.07.2009, p. 907-912.

Research output: Contribution to journal › Article › peer-review

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AU - Cooper, Russell

AU - Rahinov, Igor

AU - Yuan, Cheng

AU - Yang, Xueming

AU - Auerbach, Daniel J.

AU - Wodtke, Alec M.

N1 - Funding Information: The authors gratefully acknowledge the financial support from the Department of Energy Office of Basic Energy Sciences, under Grant No. DE-FG02-03ER15441 as well as the Partnership for International Research and Education—for Electronic Chemistry and Catalysis at Interfaces—NSF Grant No. OISE-0530268.

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AB - The authors report high resolution state resolved measurements of the translational inelasticity of HCl (v=0→0,J=0→4) colliding with a Au(111) surface at near normal incidence in the energy range of 0.28-1.27 eV. The translational inelasticity is large and indistinguishable from previous measurements for the HCl (v=2→2,J=1→5) channel. They discuss these observations in terms of an impulse approximation as well as the possible role of translational excitation of electron-hole pairs in the solid.

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Efficient translational excitation of a solid metal surface: State-to-state translational energy distributions of vibrational ground state HCl scattering from Au(111)

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