How small can a catenane be, if we consider quantum tunnelling?

Sindy Julieth Rodríguez-Sotelo, Juan Julian Santoyo-Flores, Sebastian Kozuch

Research output: Contribution to journalArticlepeer-review

Abstract

We explored the kinetic stability of the smallest possible alkane-based catenanes and pseudo-rotaxanes, focusing on their heavy atom quantum tunnelling instability. We found that the “corset effect” exerted by a ten-membered ring renders other rings unstable even under deep cryogenic conditions, where it may be taken as stable if tunnelling is neglected.

Original languageEnglish
Pages (from-to)14744-14747
Number of pages4
JournalPhysical Chemistry Chemical Physics
Volume27
Issue number28
DOIs
StatePublished - 24 Jun 2025

ASJC Scopus subject areas

  • General Physics and Astronomy
  • Physical and Theoretical Chemistry

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