Optimization of π-a isotherms to give highly efficient SHG from Langmuir-Blodgett films

H. Schwartz; P. Krief; J. Y. Becker; L. Shapiro; V. Khodorkovsky; J. T. Klug; E. Kovalev; G. Meshulam; G. Berkovic; Z. Kotler; S. Efrima

doi:10.1117/12.452070

Optimization of π-a isotherms to give highly efficient SHG from Langmuir-Blodgett films

H. Schwartz
, P. Krief
, J. Y. Becker
, L. Shapiro
, V. Khodorkovsky
, J. T. Klug
, E. Kovalev
, G. Meshulam
, G. Berkovic
, Z. Kotler
, S. Efrima

Department of Chemistry

Research output: Contribution to journal › Conference article › peer-review

1 Scopus citations

Abstract

Langmuir-Blodgett films have been prepared from amphiphilc molecules containing an indandione-based nonlinear chromophore. Study of the pressure-area (π-A) isotherm enabled us to find optimal conditions for monolayer transfer to a glass substrate. The multilayer films thus formed exhibited strong optical second harmonic generation with a bulk nonlinear co-efficient equal to the ideal value predicted by the product of the chromophore density and its known molecular hyperpolarizability.

Original language	English
Pages (from-to)	105-111
Number of pages	7
Journal	Proceedings of SPIE - The International Society for Optical Engineering
Volume	4798
DOIs	https://doi.org/10.1117/12.452070
State	Published - 1 Dec 2002
Event	Linear and Nonlinear Optics of Organic Materials II - Seattle, WA, United States Duration: 9 Jul 2002 → 11 Jul 2002

Keywords

Langmuir-Blodgett film
Organic molecules
Second harmonic generation

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Condensed Matter Physics
Computer Science Applications
Applied Mathematics
Electrical and Electronic Engineering

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10.1117/12.452070

Cite this

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title = "Optimization of π-a isotherms to give highly efficient SHG from Langmuir-Blodgett films",

abstract = "Langmuir-Blodgett films have been prepared from amphiphilc molecules containing an indandione-based nonlinear chromophore. Study of the pressure-area (π-A) isotherm enabled us to find optimal conditions for monolayer transfer to a glass substrate. The multilayer films thus formed exhibited strong optical second harmonic generation with a bulk nonlinear co-efficient equal to the ideal value predicted by the product of the chromophore density and its known molecular hyperpolarizability.",

keywords = "Langmuir-Blodgett film, Organic molecules, Second harmonic generation",

author = "H. Schwartz and P. Krief and Becker, \{J. Y.\} and L. Shapiro and V. Khodorkovsky and Klug, \{J. T.\} and E. Kovalev and G. Meshulam and G. Berkovic and Z. Kotler and S. Efrima",

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month = dec,

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doi = "10.1117/12.452070",

language = "English",

volume = "4798",

pages = "105--111",

journal = "Proceedings of SPIE - The International Society for Optical Engineering",

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note = "Linear and Nonlinear Optics of Organic Materials II ; Conference date: 09-07-2002 Through 11-07-2002",

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TY - JOUR

T1 - Optimization of π-a isotherms to give highly efficient SHG from Langmuir-Blodgett films

AU - Schwartz, H.

AU - Krief, P.

AU - Becker, J. Y.

AU - Shapiro, L.

AU - Khodorkovsky, V.

AU - Klug, J. T.

AU - Kovalev, E.

AU - Meshulam, G.

AU - Berkovic, G.

AU - Kotler, Z.

AU - Efrima, S.

PY - 2002/12/1

Y1 - 2002/12/1

N2 - Langmuir-Blodgett films have been prepared from amphiphilc molecules containing an indandione-based nonlinear chromophore. Study of the pressure-area (π-A) isotherm enabled us to find optimal conditions for monolayer transfer to a glass substrate. The multilayer films thus formed exhibited strong optical second harmonic generation with a bulk nonlinear co-efficient equal to the ideal value predicted by the product of the chromophore density and its known molecular hyperpolarizability.

AB - Langmuir-Blodgett films have been prepared from amphiphilc molecules containing an indandione-based nonlinear chromophore. Study of the pressure-area (π-A) isotherm enabled us to find optimal conditions for monolayer transfer to a glass substrate. The multilayer films thus formed exhibited strong optical second harmonic generation with a bulk nonlinear co-efficient equal to the ideal value predicted by the product of the chromophore density and its known molecular hyperpolarizability.

KW - Langmuir-Blodgett film

KW - Organic molecules

KW - Second harmonic generation

UR - https://www.scopus.com/pages/publications/0037740791

U2 - 10.1117/12.452070

DO - 10.1117/12.452070

M3 - Conference article

AN - SCOPUS:0037740791

SN - 0277-786X

VL - 4798

SP - 105

EP - 111

JO - Proceedings of SPIE - The International Society for Optical Engineering

JF - Proceedings of SPIE - The International Society for Optical Engineering

T2 - Linear and Nonlinear Optics of Organic Materials II

Y2 - 9 July 2002 through 11 July 2002

ER -

Optimization of π-a isotherms to give highly efficient SHG from Langmuir-Blodgett films

Abstract

Keywords

ASJC Scopus subject areas

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