Population transfer by multiple stimulated Raman scattering

Y. B. Band, P. S. Julienne

Research output: Contribution to journalArticlepeer-review

45 Scopus citations


We present results of density matrix calculations describing population transfer in a four level system via stimulated Raman scattering with three laser pulses whose frequencies are in (or nearly in) resonance with the transitions between the levels. A high degree of transfer to the terminal level is possible via transitions through the two intermediate excited levels, despite the large decay rates of both levels compared with the inverse of the laser pulse durations, provided that the pulse timing sequences are correctly adjusted. Hence multiple stimulated Raman scattering can be an efficient method of moving population into a given molecular level.

Original languageEnglish
Pages (from-to)5681-5685
Number of pages5
JournalJournal of Chemical Physics
Issue number8
StatePublished - 1 Jan 1991

ASJC Scopus subject areas

  • Physics and Astronomy (all)
  • Physical and Theoretical Chemistry


Dive into the research topics of 'Population transfer by multiple stimulated Raman scattering'. Together they form a unique fingerprint.

Cite this