Radionuclide Transport Simulations Supporting Proposed Borehole Waste Disposal in Israel

Katherine Carol Swager, Suzanne Michelle Bourret, Gilles Y. Bussod, Noa Balaban, Hakim Boukhalfa, Ran Calvo, Ofra Klein-BenDavid, Dolan Lucero, Itay J. Reznik, Ravid Rosenzweig, Philip H. Stauffer

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

A scientific collaboration between the U.S. and Israel is underway to assess the suitability of a potential site for subsurface radioactive waste disposal in the Negev Desert, Israel. The Negev Desert has several favorable attributes for geologic disposal, including an arid climate, a deep vadose zone, interlayered low-permeability lithologies, and carbonate rocks with high uranium-sorption potential. These features may provide a robust natural barrier to radionuclide migration. Geologic and laboratory characterization data from the Negev Desert are incorporated into multiphase flow and transport models, solved using PFLOTRAN, to aid in site characterization and risk analysis that will support decision-making for waste disposal in an intermediate-depth borehole design. The lithology with the greatest uranium sorption potential at the site is phosphorite. We use modeling to evaluate the ability of this layer to impact uranium transport around a proposed disposal borehole. The current objective of the simulations is focused on characterizing hypothetical leakage from waste canisters and subsequent uranium migration under three infiltration scenarios. Here, we describe a hydrogeologic model based on data from a local exploratory borehole and present results for uranium flow and transport simulations under varying infiltration scenarios. We find that under the current climate conditions, it is likely that uranium will remain in the near-field of the borehole for thousands of years. However, under a hypothesized extreme climate scenario representing an increase in infiltration by a factor of 300x above present-day values, uranium may break through the phosphorite layer and exit the base of the model domain (~200 m above the water table) within 1000 years. Simulation results have direct implications for the planning of nuclear waste disposal in the Negev Desert, and specifically in intermediate-depth boreholes.

Original languageEnglish
Article number166
JournalGeosciences (Switzerland)
Volume13
Issue number6
DOIs
StatePublished - 1 Jun 2023
Externally publishedYes

Keywords

  • PFLOTRAN
  • intermediate borehole disposal
  • multiphase flow
  • radionuclide transport

ASJC Scopus subject areas

  • General Earth and Planetary Sciences

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