Ultrafast two-dimensional electronic spectroscopy of millimeter-sized halide perovskite single crystals

X. Trung Nguyen; Daniel Timmer; Yevgeny Rakita; David Cahen; Antonietta de Sio; Christoph Lienau

Ultrafast two-dimensional electronic spectroscopy of millimeter-sized halide perovskite single crystals

X. Trung Nguyen
, Daniel Timmer
, Yevgeny Rakita
, David Cahen
, Antonietta de Sio
, Christoph Lienau

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Abstract

Halide perovskites (HaPs) have rapidly grown as highly promising photovoltaic materials. Despite the impressive device efficiencies, however, the fundamental mechanisms governing their unusual optoelectronic properties are still unclear [1]. In particular, the nature of their elementary optical excitations, their dynamics and interactions on ultrafast timescales are currently debated. Due to the comparatively low exciton binding energy, typically < 50 meV[2], the near-bandgap absorption in HaPs is a mixture of excitons and free carrier transitions. This makes it challenging to distinguish the contributions of these two species to the nonlinear optical spectra in experiments, in particular at room temperature.

Original language	English
Title of host publication	European Quantum Electronics Conference, EQEC_2019
Publisher	Optica Publishing Group (formerly OSA)
ISBN (Print)	9781728104690
State	Published - 1 Jan 2019
Externally published	Yes
Event	European Quantum Electronics Conference, EQEC_2019 - Munich, United Kingdom Duration: 23 Jun 2019 → 27 Jun 2019

Publication series

Name	Optics InfoBase Conference Papers
Volume	Part F143-EQEC 2019
ISSN (Electronic)	2162-2701

Conference

Conference	European Quantum Electronics Conference, EQEC_2019
Country/Territory	United Kingdom
City	Munich
Period	23/06/19 → 27/06/19

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Mechanics of Materials

Cite this

@inproceedings{4ea7c2beae364564be5f66d0691a03cd,

title = "Ultrafast two-dimensional electronic spectroscopy of millimeter-sized halide perovskite single crystals",

abstract = "Halide perovskites (HaPs) have rapidly grown as highly promising photovoltaic materials. Despite the impressive device efficiencies, however, the fundamental mechanisms governing their unusual optoelectronic properties are still unclear [1]. In particular, the nature of their elementary optical excitations, their dynamics and interactions on ultrafast timescales are currently debated. Due to the comparatively low exciton binding energy, typically < 50 meV[2], the near-bandgap absorption in HaPs is a mixture of excitons and free carrier transitions. This makes it challenging to distinguish the contributions of these two species to the nonlinear optical spectra in experiments, in particular at room temperature.",

author = "\{Trung Nguyen\}, X. and Daniel Timmer and Yevgeny Rakita and David Cahen and \{de Sio\}, Antonietta and Christoph Lienau",

note = "Publisher Copyright: {\textcopyright} 2019 IEEE; European Quantum Electronics Conference, EQEC\_2019 ; Conference date: 23-06-2019 Through 27-06-2019",

year = "2019",

month = jan,

day = "1",

language = "English",

isbn = "9781728104690",

series = "Optics InfoBase Conference Papers",

publisher = "Optica Publishing Group (formerly OSA)",

booktitle = "European Quantum Electronics Conference, EQEC\_2019",

}

Trung Nguyen, X, Timmer, D, Rakita, Y, Cahen, D, de Sio, A & Lienau, C 2019, Ultrafast two-dimensional electronic spectroscopy of millimeter-sized halide perovskite single crystals. in European Quantum Electronics Conference, EQEC_2019., 2019-eg_p_17, Optics InfoBase Conference Papers, vol. Part F143-EQEC 2019, Optica Publishing Group (formerly OSA), European Quantum Electronics Conference, EQEC_2019, Munich, United Kingdom, 23/06/19.

Ultrafast two-dimensional electronic spectroscopy of millimeter-sized halide perovskite single crystals. / Trung Nguyen, X.; Timmer, Daniel; Rakita, Yevgeny et al.
European Quantum Electronics Conference, EQEC_2019. Optica Publishing Group (formerly OSA), 2019. 2019-eg_p_17 (Optics InfoBase Conference Papers; Vol. Part F143-EQEC 2019).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Ultrafast two-dimensional electronic spectroscopy of millimeter-sized halide perovskite single crystals

AU - Trung Nguyen, X.

AU - Timmer, Daniel

AU - Rakita, Yevgeny

AU - Cahen, David

AU - de Sio, Antonietta

AU - Lienau, Christoph

PY - 2019/1/1

Y1 - 2019/1/1

N2 - Halide perovskites (HaPs) have rapidly grown as highly promising photovoltaic materials. Despite the impressive device efficiencies, however, the fundamental mechanisms governing their unusual optoelectronic properties are still unclear [1]. In particular, the nature of their elementary optical excitations, their dynamics and interactions on ultrafast timescales are currently debated. Due to the comparatively low exciton binding energy, typically < 50 meV[2], the near-bandgap absorption in HaPs is a mixture of excitons and free carrier transitions. This makes it challenging to distinguish the contributions of these two species to the nonlinear optical spectra in experiments, in particular at room temperature.

AB - Halide perovskites (HaPs) have rapidly grown as highly promising photovoltaic materials. Despite the impressive device efficiencies, however, the fundamental mechanisms governing their unusual optoelectronic properties are still unclear [1]. In particular, the nature of their elementary optical excitations, their dynamics and interactions on ultrafast timescales are currently debated. Due to the comparatively low exciton binding energy, typically < 50 meV[2], the near-bandgap absorption in HaPs is a mixture of excitons and free carrier transitions. This makes it challenging to distinguish the contributions of these two species to the nonlinear optical spectra in experiments, in particular at room temperature.

UR - https://www.scopus.com/pages/publications/85084582955

M3 - Conference contribution

AN - SCOPUS:85084582955

SN - 9781728104690

T3 - Optics InfoBase Conference Papers

BT - European Quantum Electronics Conference, EQEC_2019

PB - Optica Publishing Group (formerly OSA)

T2 - European Quantum Electronics Conference, EQEC_2019

Y2 - 23 June 2019 through 27 June 2019

ER -

Ultrafast two-dimensional electronic spectroscopy of millimeter-sized halide perovskite single crystals

Abstract

Publication series

Conference

UN SDGs

ASJC Scopus subject areas

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Cite this